Importance of Micropore–Mesopore Interfaces in Carbon Dioxide Capture by Carbon‐Based Materials
نویسندگان
چکیده
منابع مشابه
Toward carbon dioxide capture using nanoporous materials*
The development of more efficient processes for CO2 capture from the flue streams of power plants is considered a key to the reduction of greenhouse gas emissions implicated in global warming. Indeed, several U.S. and international climate change initiatives have identified the urgent need for improved materials and methods for CO2 capture. Conventional CO2 capture processes employed in power p...
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The escalating level of atmospheric carbon dioxide is one of the most pressing environmental concerns of our age. Carbon capture and storage (CCS) from large point sources such as power plants is one option for reducing anthropogenic CO(2) emissions; however, currently the capture alone will increase the energy requirements of a plant by 25-40%. This Review highlights the challenges for capture...
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In this study, bimodal meso-porous silica (UVM-7) synthesized and fabricated amino silane modified supports were characterized by powder X-ray diffraction (XRD), N2 adsorption/desorption, transmission electron microscope (TEM), elemental analysis and titration. Capacity of CO2 capture on modified bimodal pore structure silica at 70°C was calculated using breakthrough curves; and it was found th...
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Materials and processes for CO2 capture and utilisation are an essential part of a holistic approach toward a sustainable energy future. CO2 and energy are tightly intertwined as energy produced from fossil fuel combustion always generates CO2. A major environmental concern, CO2 could also become an invaluable resource for making carbon-based materials and chemicals, and a means to store energy...
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We have optimized the geometry and calculated interaction energies for over 100 different complexes of CO(2) with various combinations of electron accepting (Lewis acid) and electron donating (Lewis base) molecules. We have used the recently developed explicitly correlated coupled cluster singles doubles and perturbative triples [CCSD(T)-F12] methods and the associated VXZ-F12 (where X = D,T,Q)...
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ژورنال
عنوان ژورنال: Angewandte Chemie
سال: 2016
ISSN: 0044-8249,1521-3757
DOI: 10.1002/ange.201602226